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The many examples illustrate the concepts very well, and I particularly like the useful tips, 'common programming errors' and 'good programming practice' advice.
Surprisingly, the material is also accessible to people new to programming. There's sufficient introductory material (which experienced programmers can skip over) to allow program novices to start programming with C# - no need to start with Basic in a DOS window!
I have a few other books on C#, but this is easily the best.
I purchased Professional C# from Wrox, but I saw too many typos in the text and even worse in the code!, so I went ahead and returned it later. I decided to spend some time at the bookstore comparing books and after much deliberation this one won me. I think it was a little bit expensive but it was worth it since it includes clear explanations, visual representation of what the samples do and how they work and best of all, it covers may topics I was interested in like XML, SOAP, Web Services, ASP.NET, etc.
I even liked the two color schema (red and black) in which it is printed.